Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions

Markus Nesselberger; Sean James Ashton; Gustav Karl Henrik Wiberg; Matthias Arenz

doi:10.1063/1.4816826

Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions

Markus Nesselberger, Sean James Ashton, Gustav Karl Henrik Wiberg, Matthias Arenz

Kemisk Institut

10 Citationer (Scopus)

Abstract

We present a detailed description of the construction of an in situ electrochemical ATR-FTIR setup combined with a wall-jet electrode to investigate the electrocatalytic properties of nanoparticulate catalysts in situ under controlled mass transport conditions. The presented setup allows the electrochemical interface to be probed in combination with the simultaneous determination of reaction rates. At the same time, the high level of automation allows it to be used as a standard tool in electrocatalysis research. The performance of the setup was demonstrated by probing the oxygen reduction reaction on a platinum black catalyst in sulfuric electrolyte.

Originalsprog	Engelsk
Artikelnummer	074103
Tidsskrift	Review of Scientific Instruments
Vol/bind	84
Antal sider	7
ISSN	0034-6748
DOI	https://doi.org/10.1063/1.4816826
Status	Udgivet - jul. 2013

Adgang til dokumentet

10.1063/1.4816826

Fingeraftryk

Dyk ned i forskningsemnerne om 'Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions'. Sammen danner de et unikt fingeraftryk.

Citationsformater

Nesselberger, M., Ashton, S. J., Wiberg, G. K. H., & Arenz, M. (2013). Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions. Review of Scientific Instruments, 84, [074103]. https://doi.org/10.1063/1.4816826

Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions. / Nesselberger, Markus; Ashton, Sean James; Wiberg, Gustav Karl Henrik et al.

I: Review of Scientific Instruments, Bind 84, 074103, 07.2013.

Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › peer review

Nesselberger, M, Ashton, SJ, Wiberg, GKH & Arenz, M 2013, 'Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions', Review of Scientific Instruments, bind 84, 074103. https://doi.org/10.1063/1.4816826

Nesselberger M, Ashton SJ, Wiberg GKH, Arenz M. Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions. Review of Scientific Instruments. 2013 jul.;84:074103. doi: 10.1063/1.4816826

Nesselberger, Markus ; Ashton, Sean James ; Wiberg, Gustav Karl Henrik et al. / Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions. I: Review of Scientific Instruments. 2013 ; Bind 84.

@article{b84531b2cf464059bdf408c2a3fc1ed7,

title = "Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions",

abstract = "We present a detailed description of the construction of an in situ electrochemical ATR-FTIR setup combined with a wall-jet electrode to investigate the electrocatalytic properties of nanoparticulate catalysts in situ under controlled mass transport conditions. The presented setup allows the electrochemical interface to be probed in combination with the simultaneous determination of reaction rates. At the same time, the high level of automation allows it to be used as a standard tool in electrocatalysis research. The performance of the setup was demonstrated by probing the oxygen reduction reaction on a platinum black catalyst in sulfuric electrolyte.",

author = "Markus Nesselberger and Ashton, {Sean James} and Wiberg, {Gustav Karl Henrik} and Matthias Arenz",

year = "2013",

month = jul,

doi = "10.1063/1.4816826",

language = "English",

volume = "84",

journal = "Review of Scientific Instruments",

issn = "0034-6748",

publisher = "American Institute of Physics",

}

TY - JOUR

T1 - Design, development, and demonstration of a fully LabVIEW controlled in situ electrochemical Fourier transform infrared setup combined with a wall-jet electrode to investigate the electrochemical interface of nanoparticulate electrocatalysts under reaction conditions

AU - Nesselberger, Markus

AU - Ashton, Sean James

AU - Wiberg, Gustav Karl Henrik

AU - Arenz, Matthias

PY - 2013/7

Y1 - 2013/7

N2 - We present a detailed description of the construction of an in situ electrochemical ATR-FTIR setup combined with a wall-jet electrode to investigate the electrocatalytic properties of nanoparticulate catalysts in situ under controlled mass transport conditions. The presented setup allows the electrochemical interface to be probed in combination with the simultaneous determination of reaction rates. At the same time, the high level of automation allows it to be used as a standard tool in electrocatalysis research. The performance of the setup was demonstrated by probing the oxygen reduction reaction on a platinum black catalyst in sulfuric electrolyte.

AB - We present a detailed description of the construction of an in situ electrochemical ATR-FTIR setup combined with a wall-jet electrode to investigate the electrocatalytic properties of nanoparticulate catalysts in situ under controlled mass transport conditions. The presented setup allows the electrochemical interface to be probed in combination with the simultaneous determination of reaction rates. At the same time, the high level of automation allows it to be used as a standard tool in electrocatalysis research. The performance of the setup was demonstrated by probing the oxygen reduction reaction on a platinum black catalyst in sulfuric electrolyte.

U2 - 10.1063/1.4816826

DO - 10.1063/1.4816826

M3 - Journal article

C2 - 23902087

SN - 0034-6748

VL - 84

JO - Review of Scientific Instruments

JF - Review of Scientific Instruments

M1 - 074103

ER -