Abstract
Polarized small-angle neutron scattering studies of single-crystalline multiferroic BiFeO3 reveal a long-wavelength spin density wave generated by ∼1° spin canting of the spins out of the rotation plane of the antiferromagnetic cycloidal order. This signifies weak ferromagnetism within mesoscopic regions of dimension 0.03 microns along [11̄0], to several microns along [111], confirming a long-standing theoretical prediction. The average local magnetization is 0.06μB/Fe. Our results provide an indication of the intrinsic macroscopic magnetization to be expected in ferroelectric BiFeO3 thin films under strain, where the magnetic cycloid is suppressed.
Original language | English |
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Journal | Physical Review Letters |
Volume | 107 |
Issue number | 20 |
Pages (from-to) | 207206 |
Number of pages | 5 |
ISSN | 0031-9007 |
DOIs | |
Publication status | Published - 11 Nov 2011 |